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Research and Development of High Performance Ceramics With Structural and Functional Properties Combined

Jiang Dongliang

Strategic Study of CAE 2003, Volume 5, Issue 2, Pages 35-39

Abstract:

This paper introduces some developing trends of new materials and material sciences, such as multifunction, composite, miniaturization, low cost manufacturing and analyses the basic properties and problems of processing of high performance ceramics nowadays. The paper briefly describes some special properties, possible application fields and mass production problems of ceramics with structural and functional properties combined, such as silicon carbide, Nd doped YAG, and Sialon with rare-earth elements added. Finally, proposed several topics (including processing sciences)of such kind of multifunction materials for future research and developing.

Keywords： structural and functional properties combined high performance ceramics SiC Nd - YAG RE-Si3sub>N4sub>

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POCl3sub> diffusion for industrial Si solar cell emitter formation

Hongzhao LI,Kyung KIM,Brett HALLAM,Bram HOEX,Stuart WENHAM,Malcolm ABBOTT

Frontiers in Energy 2017, Volume 11, Issue 1, Pages 42-51 doi: 10.1007/s11708-016-0433-7

Abstract: POCl diffusion is currently the standard method for industrial n-type emitter fabrication. In this study, we present the impact of the following processing parameters on emitter formation and electrical performance: deposition gas flow ratio, drive-in temperature and duration, drive-in O flow rate, and thermal oxidation temperature. By showing their influence on the emitter doping profile and recombination activity, we provide an overall strategy for improving industrial POCl tube diffused emitters.

Keywords： POCl3sub> diffusion emitter recombination oxidation silicon

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Chemical deactivation of V

Xiaodong WU, Wenchao YU, Zhichun SI, Duan WENG

Frontiers of Environmental Science & Engineering 2013, Volume 7, Issue 3, Pages 420-427 doi: 10.1007/s11783-013-0489-0

Abstract: V O -WO /TiO catalyst was poisoned by impregnation with NH Cl, KOH and KCl solution, respectively. The catalysts were characterized by X-ray diffraction (XRD), inductively coupled plasma (ICP), N physisorption, Raman, UV-vis, NH adsorption, temperature-programmed reduction of hydrogen (H -TPR), temperature-programmed oxidation of ammonia (NH -TPO) and selective catalytic reduction of NO with ammonia (NH -SCR). The deactivation effects of poisoning agents follow the sequence of KCl>KOH>>NH Cl. The addition of ammonia chloride enlarges the pore size of the titania support, and promotes the formation of highly dispersed V=O vanadyl which improves the oxidation of ammonia and the high-temperature SCR activity. K ions are suggested to interact with vanadium and tungsten species chemically, resulting in a poor redox property of catalyst. More importantly, potassium can reduce the Br?nsted acidity of catalysts and decrease the stability of Br?nsted acid sites significantly. The more severe deactivation of the KCl-treated catalyst can be mainly ascribed to the higher amount of potassium resided on catalyst.

Keywords： V2sub>O5sub>-WO3sub>/TiO2sub> potassium chloride poisoning reducibility acid

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Covering α-Fe

Jing Gu, Hongtao Yu, Xie Quan, Shuo Chen

Frontiers of Environmental Science & Engineering 2017, Volume 11, Issue 6, doi: 10.1007/s11783-017-0957-z

Abstract: The spontaneous oxidation process of pristine silicon (Si) limits its application as photocatalyst orCovering a protection layer on Si surface is an effective approach to overcome this disadvantage.be an excellent alternative as a protection material. α-Fe O layer was deposited around each p-type Siphotogenerated-charge-separation efficiency deriving from built-in electric field at the interface between SiThe above results show an effective strategy to utilize Si material as photocatalyst or electrode in

Keywords： Si α-Fe2sub>O3sub> Photoelectrochemistry Photogenerated charge separation

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Preparation and lithium storage performances of g-C

Zhengxu BIAN, Zehua TANG, Jinfeng XIE, Junhao ZHANG, Xingmei GUO, Yuanjun LIU, Aihua YUAN, Feng ZHANG, Qinghong KONG

Frontiers in Energy 2020, Volume 14, Issue 4, Pages 759-766 doi: 10.1007/s11708-020-0810-0

Abstract: To ameliorate the volume expansion issue of silicon-based anode materials, g-C N /Si nanocomposites areIt is well known that g-C N /Si nanocomposites can not only improve the electronic transmission abilityWhen g-C N /Si electrode is evaluated, the initial discharge capacity of g-C N /Si nanocomposites isThe superior lithium storage performances benefit from the unique g-C N /Si nanostructure, which improves

Keywords： magnesium thermal reduction g-C3sub>N4sub>/Si nanocomposites volume expansion electroconductivity

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Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Frontiers of Chemical Science and Engineering 2017, Volume 11, Issue 4, Pages 586-593 doi: 10.1007/s11705-017-1659-6

Abstract: Hexagonal CePO nanorods were prepared by a precipitation method and hexagonal CePO nanowires were prepared by hydrothermal synthesis at 150 °C. Rh(NO ) was then used as a precursor for the impregnation of Rh O onto these CePO materials. The Rh O supported on the CePO nanowires was much more active for the catalytic decomposition of N O than the Rh O supported on CePO nanorods. The stability of both catalysts as a function of time on stream was studied and the influence of the co-feed (CO , O , H O or O /H O) on the N O decomposition was also investigated. The samples were characterized by N adsorption-desorption, inductively coupled plasma optical emission spectroscopy, X-ray diffraction, transmission electron microscopy, X-ray photoelectron microscopy, hydrogen temperature-programmed reduction, oxygen temperature-programmed desorption, and CO temperature-programmed desorption in order to correlate the physicochemical and catalytic properties.

Keywords： Rh2sub>O3sub> CePO4sub> N2sub>O decomposition

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Efficient CO

Yanxia Wang, Xiude Hu, Tuo Guo, Jian Hao, Chongdian Si, Qingjie Guo

Frontiers of Chemical Science and Engineering 2021, Volume 15, Issue 3, Pages 493-504 doi: 10.1007/s11705-020-1967-0

Abstract: In this work, nitrogen-doped porous carbons (NACs) were fabricated as an adsorbent by urea modification and KOH activation. The CO adsorption mechanism for the NACs was then explored. The NACs are found to present a large specific surface area (1920.72–3078.99 m ·g ) and high micropore percentage (61.60%–76.23%). Under a pressure of 1 bar, sample NAC-650-650 shows the highest CO adsorption capacity up to 5.96 and 3.92 mmol·g at 0 and 25 °C, respectively. In addition, the CO /N selectivity of NAC-650-650 is 79.93, much higher than the value of 49.77 obtained for the nonnitrogen-doped carbon AC-650-650. The CO adsorption capacity of the NAC-650-650 sample maintains over 97% after ten cycles. Analysis of the results show that the CO capacity of the NACs has a linear correlation ( = 0.9633) with the cumulative pore volume for a pore size less than 1.02 nm. The presence of nitrogen and oxygen enhances the CO /N selectivity, and pyrrole-N and hydroxy groups contribute more to the CO adsorption. Fourier transform infrared spectra analysis indicates that CO is adsorbed onto the NACs as a gas. Furthermore, the physical adsorption mechanism is confirmed by adsorption kinetic models and the isosteric heat, and it is found to be controlled by CO diffusion. The CO adsorption kinetics for NACs at room temperature and in pure CO is in accordance with the pseudo-first-order model and Avramís fractional-order kinetic model.

Keywords： porous carbon CO2sub> adsorption nitrogen-doped adsorption mechanism kinetics

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Thermodynamic Analysis and Reaction Model of Combustion Synthesis in Al-Cr2sub>O3sub> Systemwith Al2sub>O3sub> and Cr2sub>O3sub> Diluents

Zhang Yancheng,Pan Ye,Zhang Chuan

Strategic Study of CAE 2004, Volume 6, Issue 6, Pages 63-67

Abstract: lt;/sub>O3 system with AI2O3and Cr2O3 diluents were conducted, and the effects of reactionstarting temperature TO, diluents AI2O3 and Cr2O3 on the adiabatic combustion temperatureThe near linear relation between T0 and Tad was obtained

Keywords： cermet combustion synthesis Al - Cr2sub>O3sub> system thermodynamics reaction model

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In-MOF-derived In2sub>S3sub>/Bi2sub>S3sub> heterojunction for enhanced photocatalytic

Frontiers in Energy 2023, Volume 17, Issue 5, Pages 654-663 doi: 10.1007/s11708-023-0885-5

Abstract: In this paper, a broad spectrum responsive In2sub>S3sub>/Bi2sub>S3sub> heterojunctionis constructed by in-situ integrating Bi2sub>S3sub> with the In2sub>S2sub>S3sub>/Bi2sub>S3sub> heterojunction demonstrates a rate of 0.71 mmol/(g∙h), which is 2.2 and 1.7 times as much as those of In2sub>S3sub> (0.32 mmol/(g∙h) and Bi2sub>S3sub> (0.41 mmol/(g∙h)), respectively.

Keywords： photocatalytic hydrogen production wide-spectrum response metal sulfides MOFs derivative heterogeneous interfacial contact

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The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1423-1429 doi: 10.1007/s11705-023-2315-y

Abstract: To enhance the stability, the traditional carrier Al2sub>O3sub> with a small amount, wasintroduced into Pb/SiO2sub> catalyst in this study.It has been proved that Al2sub>O3sub> can inhibit the reduction of PbO, and weaken theAs a result, 3Al15Pb/SiO2sub> catalyst exhibits a much higher stability up to more than 150 h.>2sub>O3sub> addition was also proposed.

Keywords： Pb/SiO2sub> Al2sub>O3sub> propane dehydrogenation propene stability

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Synthesis and anticancer activity of (+)-nopinone-based 2-amino-3-cyanopyridines

Shengliang LIAO,Shibin SHANG,Minggui SHEN,Xiaoping RAO,Hongyan SI,Jie SONG,Zhanqian SONG

Frontiers of Agricultural Science and Engineering 2015, Volume 2, Issue 4, Pages 335-340 doi: 10.15302/J-FASE-2015079

Abstract: Twelve (+)-nopinone-based 2-amino-3-cyanopyridines 4a–l were synthesized from (–)-β-pinene.

Keywords： b-pinene nopinone synthesis 2-amino-3-cyanopyridine anticancer

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Is atmospheric oxidation capacity better in indicating tropospheric O formation?

Frontiers of Environmental Science & Engineering 2022, Volume 16, Issue 5, doi: 10.1007/s11783-022-1544-5

Abstract: ListItem>

● This study summarizes and evaluates different approaches that indicate O3sub> formation.

Keywords： O3sub> AOC O3sub> formation regime

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acid anions on highly efficient Ce-based catalysts for selective catalytic reduction of NO with NH3sub>

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 10, Pages 1399-1411 doi: 10.1007/s11705-023-2345-5

Abstract: 3sub>) were synthesized and used for the selective catalytic reduction (SCR) of NO by NH3NH3sub>-SCR performances were conducted in the temperature range of 80 to 400 °C.> Ce2sub>(SO4sub>)3sub>, which is in agreement with their abilities of NH3sub>4sub>^3–, VO4sub>^3– and SO4sub>^2–2sub> for Ce2sub>(SO4sub>)3sub>.

Keywords： CePO4sub> CeVO4sub> Ce2sub>(SO4sub>)3sub> selective catalytic reduction

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On the monolayer dispersion behavior of Co3sub>O4sub> on HZSM-5 support: designing applicable

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 11, Pages 1741-1754 doi: 10.1007/s11705-023-2332-x

Abstract: Based on monolayer dispersion theory, Co3sub>O4sub>/ZSM-5 catalysts with different loadingsCo3sub>O4sub> can spontaneously disperse on HZSM-5 support with a monolayer dispersionBelow the monolayer dispersion threshold, Co3sub>O4sub> is finely dispersed as sub-monolayersHowever, the formation of crystalline Co3sub>O4sub> above the capacity is harmful to thecapacity amount of Co3sub>O4sub> onto HZSM-5 support.

Keywords： Co3sub>O4sub>/ZSM-5 NOxsub>-SCR by NH3sub> monolayer dispersionthreshold effect surface acid sites surface active O2sub>^– anions

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Feasibility study of plasma sprayed Al2sub>O3sub> coatings as diffusion barrier on CFC

Kirsten BOBZIN, Lidong ZHAO, Nils KOPP, Thomas WARDA

Frontiers of Mechanical Engineering 2012, Volume 7, Issue 4, Pages 371-375 doi: 10.1007/s11465-012-0339-y

Abstract: Within this study the feasibility of plasma sprayed Al2sub>O3sub> coatings as diffusionAl2sub>O3sub> coatings were prepared by air plasma spraying (APS).The results showed that Al2sub>O3sub> could be well deposited onto CFC substrates.temperature of 1270°C, crack network formed within the coating, showing that the plasma sprayed Al2sub>O3sub> coatings are limited regarding to their application temperatures as diffusion

Keywords： diffusion barrier coatings CFC plasma spraying microstructure Al2sub>O3sub>

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Title Author Date Type Operation

Research and Development of High Performance Ceramics With Structural and Functional Properties Combined

Jiang Dongliang

Journal Article

POCl3sub> diffusion for industrial Si solar cell emitter formation

Hongzhao LI,Kyung KIM,Brett HALLAM,Bram HOEX,Stuart WENHAM,Malcolm ABBOTT

Journal Article

Chemical deactivation of V

Xiaodong WU, Wenchao YU, Zhichun SI, Duan WENG

Journal Article

Covering α-Fe

Jing Gu, Hongtao Yu, Xie Quan, Shuo Chen

Journal Article

Preparation and lithium storage performances of g-C

Zhengxu BIAN, Zehua TANG, Jinfeng XIE, Junhao ZHANG, Xingmei GUO, Yuanjun LIU, Aihua YUAN, Feng ZHANG, Qinghong KONG

Journal Article

Rh2sub>O3sub>/hexagonal CePO4sub> nanocatalysts for N2sub>O decomposition

Huan Liu, Zhen Ma

Journal Article

Efficient CO

Yanxia Wang, Xiude Hu, Tuo Guo, Jian Hao, Chongdian Si, Qingjie Guo

Journal Article

Thermodynamic Analysis and Reaction Model of Combustion Synthesis in Al-Cr2sub>O3sub> Systemwith Al2sub>O3sub> and Cr2sub>O3sub> Diluents

Zhang Yancheng,Pan Ye,Zhang Chuan

Journal Article

In-MOF-derived In2sub>S3sub>/Bi2sub>S3sub> heterojunction for enhanced photocatalytic

Journal Article

The stabilization effect of Al2sub>O3sub> on unconventional Pb/SiO2sub> catalyst

Journal Article

Synthesis and anticancer activity of (+)-nopinone-based 2-amino-3-cyanopyridines

Shengliang LIAO,Shibin SHANG,Minggui SHEN,Xiaoping RAO,Hongyan SI,Jie SONG,Zhanqian SONG

Journal Article

Is atmospheric oxidation capacity better in indicating tropospheric O formation?

Journal Article

acid anions on highly efficient Ce-based catalysts for selective catalytic reduction of NO with NH3sub>

Journal Article

On the monolayer dispersion behavior of Co3sub>O4sub> on HZSM-5 support: designing applicable

Journal Article

Feasibility study of plasma sprayed Al2sub>O3sub> coatings as diffusion barrier on CFC

Kirsten BOBZIN, Lidong ZHAO, Nils KOPP, Thomas WARDA

Journal Article

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